Bob Dole and Sam Donaldson were both members on an alumni board for Kappa Sigma and, from what I've heard, keep tabs on how things are going in the fraternity. Dole spoke at the University of Arizona house when he was campaigning. Cowboys owner Jerry Jones has also assisted the fraternity at times from what I understand.
There's an actor who spoke at Conclave when I went in 2001, but I can't remember his name...seems he was at least marginally famous though, maybe someone can help me out.
Some of the other famous members (Rick Barry for one) did bit parts in rush videos that the fraternity put out.
I'm probably missing some, but those are the ones that come to mind.
ETA: Nice job on the mention of Redford as a Kappa Sig...I often forget that he's a brother.
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