I know DKE has a bunch, one of which I think is cool was Theodore Roosevelt. I don't know what site would have a listing for them, but I found these guys listed at a link from greekpages.com:
Kappa Alpha Order -- J. Edgar Hoover (FBI Director)
Lambda Chi Alpha -- Harry Truman (U.S. President)
Tau Kappa Epsilon -- Ronald Reagan (U.S. President)
Sigma Chi -- Barry Goldwater (Congressman) and Grover Clevland (U.S. President)
Kappa Sigma -- Bob Dole & Estes Kefauver
Pi Beta Phi (sorority) -- Margaret Truman Daniel?? (Daughter of Harry Truman)
Phi Gamma Delta (FIJI) -- Calvin Coolidge (U.S. President) and Newton Baker??2 (U.S. Secretary of War, 1916-1921)
Phi Delta Theta -- Adlai Stevenson (U.S. Vice-President)
Sigma Nu -- Lloyd Benson (Secretary of the Treasury)
Alpha Chi Rho -- Alphonse D'Amato (U.S. Senator)
Phi Kappa Psi -- Woodrow Wilson (U.S. President)
Sigma Alpha Epsilon -- William McKinley (U.S. President)
Phi Kappa Theta -- John F. Kennedy (U.S. President)
AXPAlum
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