If you can, get your hands on a Baird's Manual, or, I recall seeing this in From Here to Fraternity (out of publication for some time now) - but U Illinois and Illinois State had the largest number of chapters for a single campus (if I remember numbers right, something like 50+ fraternity chapters at each school, not sure of sorority numbers).
From personal observation, Cal Berkeley has a large greek system in number of chapters as well, as does UCLA and USC.
If you're looking for a percentage of students at a campus who are greek, the best way to determine that would be to contact campus Greek Life Directors for specifics.
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