My favorite color happens to be orange, but since that's not an option...
I tend to like unique color combinations. The ones that catch my eye are:
Alpha Gamma Delta - red, buff, green
Alpha Phi - silver, bordeaux
Alpha Xi Delta - light blue, dark blue, gold
Delta Delta Delta - silver, gold, cerulean blue
Delta Gamma - bronze, pink, blue
Pi Beta Phi - wine, silver blue
And while this combination isn't particularly "unique", it's very classy:
Kappa Kappa Gamma - light blue, dark blue
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