I imagine that belonging to a GLO is less of a prerequisite than experience in education. Depending on the school's interpretation and the responsibilities, being Greek may certainly provide some advantages.
I think that every school has a different expectation of what a Greek Life advisor should be/do. In addition to working in Student Affairs, there may be job openings for house advisors, etc. Being Greek would enhance your familiarity with the basics of Greek life, but in my college experience working in Student Government, sorority chapter officer, etc., most of the work is pretty much administrative as opposed to counseling.
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